Control of visual appearance with disordered plasmonic resonant metasurfaces
Idioma
en
Communication dans un congrès
Este ítem está publicado en
SPP 2023 - The International Conference on Surface Plasmon Photonics 10, 2023-05-21, Houston, TX,.
Resumen en inglés
A longstanding and fundamental ambition of waves science is the achievement of materials with prescribed optical properties and targeted far-field responses. Notably, light manipulation by means of micro- and nanostructured ...Leer más >
A longstanding and fundamental ambition of waves science is the achievement of materials with prescribed optical properties and targeted far-field responses. Notably, light manipulation by means of micro- and nanostructured metasurfaces has found fertile ground in the control and generation of colors and, most recently, unusual visual appearance. Be they disordered, or precisely organized, metasurfaces composed of arrays of Mie, plasmonic or Fabry-Perot nanoresonators offer several degrees of freedom for engineering visual appearance design. Curiously, most of the attention has gone to overall chromatic properties andmany important aspects that determine the integral visual appearance of a surface have been largely ignored.Quantitatively retrieving the visual appearance of metasurfaces requires advanced knowledge of the nanoscale resonances, mesoscale interferences and macroscale light transport defining the bidirectional reflectance distribution function (BRDF). This problem is inherently multidimensional and complex; hence brute-force full-wave electromagnetic analysis is not viable.In this context, we present an interpretive, intuitive and accurate modal-based tool that unveils the main physical mechanisms impacting the color and visual appearance of complex metasurfaces. We implement, test, and validate our tool for disordered colloidal monolayers of plasmonic silver nanoparticles deposited on a reflective substrate coated with a submicrometric dielectric spacer. Our approach successfully predicts and intuitively explains that metasurfaces combining plasmonic and Fabry-Perot resonances offer uncommon iridescent visual appearance not observed with natural nanostructures or thin-film interferences. The model also clarifies the remarkable resilience of the iridescent metasurfaces to size and shape polydispersity of the plasmonicnanoresonators. Fabrication flexibility is essential for real applications of plasmonic metasurfaces, as it may result in a strong reduction of manufacturing costs for large-scale coatings production.We expect this work to inspire and motivate further metasurface designs exhibiting complex visual appearances that are traditionally difficult to predict and assess.< Leer menos
Proyecto ANR
Surfaces nanostructurées complexes pour la conception de l'apparence visuelle - ANR-19-CE09-0014
Orígen
Importado de HalCentros de investigación