AVRILLER, Rémi; SOUTO, R; MARTIN-RODERO, A.; YEYATI, A

doi:10.1103/PhysRevB.99.121403

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AVRILLER, Rémi
Laboratoire Ondes et Matière d'Aquitaine [LOMA]

SOUTO, R
Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center [IFIMAC]

MARTIN-RODERO, A.
Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center [IFIMAC]

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Physical Review B: Condensed Matter and Materials Physics (1998-2015). 2019-03-05, vol. 99, n° 121403

American Physical Society

Resumen en inglés

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across the junction undergo damped oscillations towards the steady-state. We assign the former to the onset of electron tunneling events assisted by vibron-emission. The time-dependent build-up of electron-hole correlations is revealed as a departure of the charge-transfer statistics from the generalized-binomial one after a critical time tc. The phonon-back action on the tunneling electrons is shown to amplify and accelerate this build-up mechanism.< Leer menos

Palabras clave en inglés

Molecular electronics

Electron-phonon interactions

Time-dependent electronic transport

DOI

http://dx.doi.org/10.1103/PhysRevB.99.121403

Proyecto ANR

Réactions Chimiques, Transfert de Charges et d'Energie en Cavité Electromagnétique

Orígen

Importado de Hal

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Laboratoire Ondes et Matière d'Aquitaine (LOMA) - UMR 5798