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Influence of Surface Chemistry of Fiber and Lignocellulosic Materials on Adhesion Properties with Polybutylene Succinate at Nanoscale

dc.rights.licenseopenen_US
dc.contributor.authorMARCUELLO, Carlos
dc.contributor.authorCHABBERT, Brigitte
dc.contributor.authorBERZIN, Francoise
dc.contributor.authorBERCU, Nicolas
hal.structure.identifierChimie et Biologie des Membranes et des Nanoobjets [CBMN]
dc.contributor.authorMOLINARI, Michael
dc.contributor.authorAGUIE-BEGHIN, Veronique
dc.date.accessioned2024-04-24T09:18:17Z
dc.date.available2024-04-24T09:18:17Z
dc.date.issued2023-03-18
dc.identifier.issn1996-1944en_US
dc.identifier.urihttps://oskar-bordeaux.fr/handle/20.500.12278/199297
dc.description.abstractEnThe production of bio-based composites with enhanced characteristics constitutes a strategic action to minimize the use of fossil fuel resources. The mechanical performances of these materials are related to the specific properties of their components, as well as to the quality of the interface between the matrix and the fibers. In a previous research study, it was shown that the polarity of the matrix played a key role in the mechanisms of fiber breakage during processing, as well as on the final properties of the composite. However, some key questions remained unanswered, and new investigations were necessary to improve the knowledge of the interactions between a lignocellulosic material and a polar matrix. In this work, for the first time, atomic force microscopy based on force spectroscopy measurements was carried out using functionalized tips to characterize the intermolecular interactions at the single molecule level, taking place between poly(butylene succinate) and four different plant fibers. The efficiency of the tip functionalization was checked out by scanning electron microscopy and energy-dispersive X-ray spectroscopy, whereas the fibers chemistry was characterized by Fourier-transform infrared spectroscopy. Larger interactions at the nanoscale level were found between the matrix and hypolignified fibers compared to lignified ones, as in control experiments on single lignocellulosic polymer films. These results could significantly aid in the design of the most appropriate composite composition depending on its final use.
dc.language.isoENen_US
dc.rights.urihttp://creativecommons.org/licenses/by/
dc.subject.enintermolecular interactions
dc.subject.enplant fibers
dc.subject.enlignocellulosic films
dc.subject.enpolybutylene succinate (PBS)
dc.subject.enatomic force microscopy
dc.subject.enforce spectroscopy
dc.subject.enfunctionalization
dc.subject.eninfrared spectroscopy
dc.title.enInfluence of Surface Chemistry of Fiber and Lignocellulosic Materials on Adhesion Properties with Polybutylene Succinate at Nanoscale
dc.typeArticle de revueen_US
dc.identifier.doi10.3390/ma16062440en_US
dc.subject.halChimieen_US
dc.subject.halSciences de l'ingénieur [physics]en_US
bordeaux.journalMaterialsen_US
bordeaux.page2440en_US
bordeaux.volume16en_US
bordeaux.hal.laboratoriesCBMN : Chimie & de Biologie des Membranes & des Nano-objets - UMR 5248en_US
bordeaux.issue6en_US
bordeaux.institutionUniversité de Bordeauxen_US
bordeaux.institutionBordeaux INPen_US
bordeaux.institutionCNRSen_US
bordeaux.peerReviewedouien_US
bordeaux.inpressnonen_US
bordeaux.import.sourcehal
hal.identifierhal-04289226
hal.version1
hal.popularnonen_US
hal.audienceInternationaleen_US
hal.exportfalse
workflow.import.sourcehal
dc.rights.ccPas de Licence CCen_US
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Materials&rft.date=2023-03-18&rft.volume=16&rft.issue=6&rft.spage=2440&rft.epage=2440&rft.eissn=1996-1944&rft.issn=1996-1944&rft.au=MARCUELLO,%20Carlos&CHABBERT,%20Brigitte&BERZIN,%20Francoise&BERCU,%20Nicolas&MOLINARI,%20Michael&rft.genre=article


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