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What is in the fish? Collaborative trial in suspect and non-target screening of organic micropollutants using LC- and GC-HRMS

dc.rights.licenseopenen_US
dc.contributor.authorDÜRIG, Wiebke
dc.contributor.authorLINDBLAD, Sofia
dc.contributor.authorGOLOVKO, Oksana
dc.contributor.authorGKOTSIS, Georgios
dc.contributor.authorAALIZADEH, Reza
dc.contributor.authorNIKA, Maria-Christina
dc.contributor.authorTHOMAIDIS, Nikolaos
dc.contributor.authorALYGIZAKIS, Nikiforos A
dc.contributor.authorPLASSMANN, Merle
dc.contributor.authorHAGLUND, Peter
dc.contributor.authorFU, Qiuguo
dc.contributor.authorHOLLENDER, Juliane
dc.contributor.authorCHAKER, Jade
dc.contributor.authorDAVID, Arthur
dc.contributor.authorKUNKEL, Uwe
dc.contributor.authorMACHERIUS, André
dc.contributor.authorBELOVA, Lidia
dc.contributor.authorPOMA, Giulia
dc.contributor.authorPREUD'HOMME, Hugues
dc.contributor.authorMUNSCHY, Catherine
dc.contributor.authorAMINOT, Yann
dc.contributor.authorJAEGER, Carsten
dc.contributor.authorLISEC, Jan
dc.contributor.authorHANSEN, Martin
dc.contributor.authorVORKAMP, Katrin
dc.contributor.authorZHU, Linyan
dc.contributor.authorCAPPELLI, Francesca
dc.contributor.authorROSCIOLI, Claudio
dc.contributor.authorVALSECCHI, Sara
dc.contributor.authorBAGNATI, Renzo
dc.contributor.authorGONZÁLEZ, Belén
dc.contributor.authorPRIETO, Ailette
dc.contributor.authorZULOAGA, Olatz
dc.contributor.authorGIL-SOLSONA, Ruben
dc.contributor.authorGAGO-FERRERO, Pablo
dc.contributor.authorRODRIGUEZ-MOZAZ, Sara
hal.structure.identifierEnvironnements et Paléoenvironnements OCéaniques [EPOC]
dc.contributor.authorBUDZINSKI, Hélène
ORCID: 0000-0003-1028-9154
IDREF: 070478090
hal.structure.identifierEnvironnements et Paléoenvironnements OCéaniques [EPOC]
dc.contributor.authorDEVIER, Marie-Helene
dc.contributor.authorDIERKES, Georg
dc.contributor.authorBOULARD, Lise
dc.contributor.authorJACOBS, Griet
dc.contributor.authorVOORSPOELS, Stefan
dc.contributor.authorRÜDEL, Heinz
dc.contributor.authorAHRENS, Lutz
dc.date.accessioned2024-08-27T11:56:13Z
dc.date.available2024-08-27T11:56:13Z
dc.date.issued2023-11-01
dc.identifier.issn1873-6750en_US
dc.identifier.urihttps://oskar-bordeaux.fr/handle/20.500.12278/201321
dc.description.abstractEnA collaborative trial involving 16 participants from nine European countries was conducted within the NORMAN network in efforts to harmonise suspect and non-target screening of environmental contaminants in whole fish samples of bream (Abramis brama). Participants were provided with freeze-dried, homogenised fish samples from a contaminated and a reference site, extracts (spiked and non-spiked) and reference sample preparation protocols for liquid chromatography (LC) and gas chromatography (GC) coupled to high resolution mass spectrometry (HRMS). Participants extracted fish samples using their in-house sample preparation method and/or the protocol provided. Participants correctly identified 9-69 % of spiked compounds using LC-HRMS and 20-60 % of spiked compounds using GC-HRMS. From the contaminated site, suspect screening with participants' own suspect lists led to putative identification of on average ∼145 and ∼20 unique features per participant using LC-HRMS and GC-HRMS, respectively, while non-target screening identified on average ∼42 and ∼56 unique features per participant using LC-HRMS and GC-HRMS, respectively. Within the same sub-group of sample preparation method, only a few features were identified by at least two participants in suspect screening (16 features using LC-HRMS, 0 features using GC-HRMS) and non-target screening (0 features using LC-HRMS, 2 features using GC-HRMS). The compounds identified had log octanol/water partition coefficient (K) values from -9.9 to 16 and mass-to-charge ratios (m/z) of 68 to 761 (LC-HRMS and GC-HRMS). A significant linear trend was found between log K and m/z for the GC-HRMS data. Overall, these findings indicate that differences in screening results are mainly due to the data analysis workflows used by different participants. Further work is needed to harmonise the results obtained when applying suspect and non-target screening approaches to environmental biota samples.
dc.language.isoENen_US
dc.rightsAttribution 3.0 United States*
dc.rights.urihttp://creativecommons.org/licenses/by/3.0/us/*
dc.subject.enAnimals
dc.subject.enHumans
dc.subject.enEnvironmental Monitoring
dc.subject.enGas Chromatography-Mass Spectrometry
dc.subject.enChromatography
dc.subject.enLiquid
dc.subject.enMass Spectrometry
dc.subject.enFishes
dc.title.enWhat is in the fish? Collaborative trial in suspect and non-target screening of organic micropollutants using LC- and GC-HRMS
dc.title.alternativeEnviron Inten_US
dc.typeArticle de revueen_US
dc.identifier.doi10.1016/j.envint.2023.108288en_US
dc.identifier.pubmed37918065en_US
bordeaux.journalEnvironment Internationalen_US
bordeaux.page108288en_US
bordeaux.volume181en_US
bordeaux.hal.laboratoriesEPOCen_US
bordeaux.institutionUniversité de Bordeauxen_US
bordeaux.institutionCNRSen_US
bordeaux.teamLPTCen_US
bordeaux.peerReviewedouien_US
bordeaux.inpressnonen_US
bordeaux.import.sourcepubmed
hal.popularnonen_US
hal.audienceInternationaleen_US
hal.exportfalse
workflow.import.sourcepubmed
dc.rights.ccCC BYen_US
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Environment%20International&rft.date=2023-11-01&rft.volume=181&rft.spage=108288&rft.epage=108288&rft.eissn=1873-6750&rft.issn=1873-6750&rft.au=D%C3%9CRIG,%20Wiebke&LINDBLAD,%20Sofia&GOLOVKO,%20Oksana&GKOTSIS,%20Georgios&AALIZADEH,%20Reza&rft.genre=article


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