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Divanillin-Based Polyazomethines: Toward Biobased and Metal-Free π-Conjugated Polymers

dc.rights.licenseopen
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorGARBAY, Guillaume
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorGIRAUD, Lauriane
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorGALI, Sai Manoj
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorHADZIIOANNOU, Georges
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorGRAU, Etienne
IDREF: 187909261
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorGRELIER, Stéphane
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorCLOUTET, Eric
IDREF: 151048681
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorCRAMAIL, Henri
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies
dc.contributor.authorBROCHON, Cyril
dc.date2020
dc.date.accessioned2020
dc.date.available2020
dc.date.issued2020
dc.identifier.issn2470-1343
dc.identifier.urihttps://oskar-bordeaux.fr/handle/20.500.12278/19721
dc.description.abstractEnDivanillin was synthesized in high yield and purity using Laccase from Trametes versicolor. It was then pol-ymerized with Benzene-1,4-diamine and 2,7-diaminocarbazole to form polyazomethines. Polymerizations were performed under microwave irradiation and without transition-metal based catalyst. These bio-based conjugated polyazomethines present a broad fluorescence spectrum ranging from 400 to 600 nm. Depending on the co-monomer used, polyazomethines with molar masses around 10 kg.mol-1 and with electronic gaps ranging from 2.66 to 2.85 eV were obtained. Furthermore, TD-DFT calculations were performed to corroborate experimental results.
dc.language.isoen
dc.publisherACS Publications
dc.subject.enPolyazomethines
dc.subject.enCarbazole
dc.subject.enDivanillin
dc.title.enDivanillin-Based Polyazomethines: Toward Biobased and Metal-Free π-Conjugated Polymers
dc.typeArticle de revue
dc.identifier.doi10.1021/acsomega.9b04181
dc.subject.halChimie/Polymères
bordeaux.journalACS Omega
bordeaux.hal.laboratoriesLaboratoire de Chimie des Polymères Organiques (LCPO) - UMR 5629*
bordeaux.institutionBordeaux INP
bordeaux.institutionUniversité de Bordeaux
bordeaux.peerReviewedoui
hal.identifierhal-02499195
hal.version1
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-02499195v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=ACS%20Omega&rft.date=2020&rft.eissn=2470-1343&rft.issn=2470-1343&rft.au=GARBAY,%20Guillaume&GIRAUD,%20Lauriane&GALI,%20Sai%20Manoj&HADZIIOANNOU,%20Georges&GRAU,%20Etienne&rft.genre=article


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