The dark exciton ground state promotes photon-pair emission in individual perovskite nanocrystals
hal.structure.identifier | Laboratoire Photonique, Numérique et Nanosciences [LP2N] | |
dc.contributor.author | TAMARAT, Philippe | |
hal.structure.identifier | Laboratoire Photonique, Numérique et Nanosciences [LP2N] | |
dc.contributor.author | HOU, Lei | |
hal.structure.identifier | Laboratoire Photonique, Numérique et Nanosciences [LP2N] | |
dc.contributor.author | TREBBIA, Jean-Baptiste | |
hal.structure.identifier | Swiss Federal Laboratories for Materials Science and Technology [Dübendorf] [EMPA] | |
hal.structure.identifier | Department of Chemistry and Applied Biosciences [ETH Zürich] [D-CHAB] | |
dc.contributor.author | SWARNKAR, Abhishek | |
hal.structure.identifier | Institut d’Électronique, de Microélectronique et de Nanotechnologie - UMR 8520 [IEMN] | |
hal.structure.identifier | Physique - IEMN [PHYSIQUE - IEMN] | |
dc.contributor.author | BIADALA, Louis | |
hal.structure.identifier | Laboratoire Ondes et Matière d'Aquitaine [LOMA] | |
dc.contributor.author | LOUYER, Yann | |
hal.structure.identifier | Swiss Federal Laboratories for Materials Science and Technology [Dübendorf] [EMPA] | |
dc.contributor.author | BODNARCHUK, Maryna | |
hal.structure.identifier | Swiss Federal Laboratories for Materials Science and Technology [Dübendorf] [EMPA] | |
hal.structure.identifier | Department of Chemistry and Applied Biosciences [ETH Zürich] [D-CHAB] | |
dc.contributor.author | KOVALENKO, Maksym | |
hal.structure.identifier | Institut des Fonctions Optiques pour les Technologies de l'informatiON [FOTON] | |
dc.contributor.author | EVEN, Jacky | |
hal.structure.identifier | Laboratoire Photonique, Numérique et Nanosciences [LP2N] | |
dc.contributor.author | LOUNIS, Brahim | |
dc.date.issued | 2020-11-26 | |
dc.identifier.issn | 2041-1723 | |
dc.description.abstractEn | Cesium lead halide perovskites exhibit outstanding optical and electronic properties for a wide range of applications in optoelectronics and for light-emitting devices. Yet, the physics of the band-edge exciton, whose recombination is at the origin of the photoluminescence, is not elucidated. Here, we unveil the exciton fine structure of individual cesium lead iodide perovskite nanocrystals and demonstrate that it is governed by the electron-hole exchange interaction and nanocrystal shape anisotropy. The lowest-energy exciton state is a long-lived dark singlet state, which promotes the creation of biexcitons at low temperatures and thus correlated photon pairs. These bright quantum emitters in the near-infrared have a photon statistics that can readily be tuned from bunching to antibunching, using magnetic or thermal coupling between dark and bright exciton sublevels. | |
dc.description.sponsorship | University of Bordeaux Graduate Scholl in Light Sciences & Technologies - ANR-17-EURE-0027 | |
dc.language.iso | en | |
dc.publisher | Nature Publishing Group | |
dc.title.en | The dark exciton ground state promotes photon-pair emission in individual perovskite nanocrystals | |
dc.type | Article de revue | |
dc.identifier.doi | 10.1038/s41467-020-19740-7 | |
dc.subject.hal | Physique [physics] | |
dc.subject.hal | Physique [physics]/Physique Quantique [quant-ph] | |
bordeaux.journal | Nature Communications | |
bordeaux.page | 6001 | |
bordeaux.volume | 11 | |
bordeaux.issue | 1 | |
bordeaux.peerReviewed | oui | |
hal.identifier | hal-03015064 | |
hal.version | 1 | |
hal.popular | non | |
hal.audience | Internationale | |
hal.origin.link | https://hal.archives-ouvertes.fr//hal-03015064v1 | |
bordeaux.COinS | ctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Nature%20Communications&rft.date=2020-11-26&rft.volume=11&rft.issue=1&rft.spage=6001&rft.epage=6001&rft.eissn=2041-1723&rft.issn=2041-1723&rft.au=TAMARAT,%20Philippe&HOU,%20Lei&TREBBIA,%20Jean-Baptiste&SWARNKAR,%20Abhishek&BIADALA,%20Louis&rft.genre=article |
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