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Toward molecular 4f single-ion magnet qubits

hal.structure.identifierCentre de recherches Paul Pascal [CRPP]
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorPEDERSEN, Kasper S.
hal.structure.identifierSchool of Chemistry and Photon Science Institute
dc.contributor.authorARICIU, Ana-Maria
hal.structure.identifierSchool of Chemistry and Photon Science Institute
dc.contributor.authorMCADAMS, Simon
hal.structure.identifierDepartment of Chemistry [Copenhagen]
dc.contributor.authorWEIHE, Høgni
hal.structure.identifierDepartment of Chemistry [Copenhagen]
dc.contributor.authorBENDIX, Jesper
hal.structure.identifierSchool of Chemistry and Photon Science Institute
dc.contributor.authorTUNA, Floriana
hal.structure.identifierDepartment of Chemistry [Copenhagen]
dc.contributor.authorPILIGKOS, Stergios
dc.date.issued2016-05-11
dc.identifier.issn0002-7863
dc.description.abstractEnQuantum coherence is detected in the 4f single-ion magnet (SIM) Yb(trensal), by isotope selective pulsed EPR spectroscopy on an oriented single crystal. At X-band, the spin-lattice relaxation (T1) and phase memory (Tm) times are found to be independent of the nuclei bearing, or not, a nuclear spin. The observation of Rabi oscillations of the spin echo demonstrates the possibility to coherently manipulate the system for more than 70 rotations. This renders Yb(trensal), a sublimable and chemically modifiable SIM, an excellent candidate for quantum information processing.
dc.language.isoen
dc.publisherAmerican Chemical Society
dc.title.enToward molecular 4f single-ion magnet qubits
dc.typeArticle de revue
dc.identifier.doi10.1021/jacs.6b02702
dc.subject.halChimie/Matériaux
bordeaux.journalJournal of the American Chemical Society
bordeaux.page5801-5804
bordeaux.volume138
bordeaux.issue18
bordeaux.peerReviewedoui
hal.identifierhal-01321193
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-01321193v1
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