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Main-chain poly(fullerene) multiblock copolymers as organic photovoltaic donor-acceptors and stabilizers
dc.rights.license | open | |
hal.structure.identifier | Laboratoire de l'intégration, du matériau au système [IMS] | |
dc.contributor.author | RAÏSSI, Mahfoudh | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
dc.contributor.author | EROTHU, Harikrishna | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
dc.contributor.author | IBARBOURE, Emmanuel | |
hal.structure.identifier | Laboratoire de l'intégration, du matériau au système [IMS] | |
dc.contributor.author | BEJBOUJI, Habiba | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
dc.contributor.author | CRAMAIL, Henri | |
hal.structure.identifier | Team 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
dc.contributor.author | CLOUTET, Eric
IDREF: 151048681 | |
hal.structure.identifier | Laboratoire de l'intégration, du matériau au système [IMS] | |
dc.contributor.author | VIGNAU, Laurence | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
hal.structure.identifier | Institut des sciences analytiques et de physico-chimie pour l'environnement et les materiaux [IPREM] | |
dc.contributor.author | HIORNS, Roger C. | |
dc.date.accessioned | 2020 | |
dc.date.available | 2020 | |
dc.date.issued | 2017 | |
dc.identifier.issn | 2050-7488 | |
dc.identifier.uri | https://oskar-bordeaux.fr/handle/20.500.12278/20123 | |
dc.description.abstractEn | A multi-block copolymer based on main-chain fullerene repeating units is used in org. photovoltaic devices for the first time. A poly(fullerene) (PFDP) is linked at the chain-ends to poly(3-hexylthiophene) (P3HT) to give poly[poly(3-hexylthiophene)-block-poly{([1,4]-fullerene)-alt-[1,4-dimethylene-2,5-bis(cyclohexylmethyl ether)phenylene]}] (P3HT-b-PFDP). While normal devices give poor results, inverted architectures result in near 50-fold improvements in performances to a block copolymer efficiency of 2.8% for this novel system. PFDP-b-P3HT is also employed as an additive to P3HT:PCBM bulk heterojunction devices and demonstrates increases from 3.6% to 4.2%, and remarkably gives a stable flat-line efficiency over the time studied. | |
dc.language.iso | en | |
dc.publisher | Royal Society of Chemistry | |
dc.subject.en | photovoltaic | |
dc.subject.en | fullerene | |
dc.subject.en | copolymer | |
dc.title.en | Main-chain poly(fullerene) multiblock copolymers as organic photovoltaic donor-acceptors and stabilizers | |
dc.type | Article de revue | |
dc.identifier.doi | 10.1039/C7TA01980G | |
dc.subject.hal | Chimie/Polymères | |
bordeaux.journal | Journal of Materials Chemistry A | |
bordeaux.page | 7533-7544 | |
bordeaux.volume | 5 | |
bordeaux.hal.laboratories | Laboratoire de Chimie des Polymères Organiques (LCPO) - UMR 5629 | * |
bordeaux.issue | 16 | |
bordeaux.institution | Bordeaux INP | |
bordeaux.institution | Université de Bordeaux | |
bordeaux.peerReviewed | oui | |
hal.identifier | hal-01505554 | |
hal.version | 1 | |
hal.origin.link | https://hal.archives-ouvertes.fr//hal-01505554v1 | |
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