High Performance All-Polymer Photodetector Comprising a Donor–Acceptor–Acceptor Structured Indacenodithiophene–Bithieno[3,4- c ]Pyrroletetrone Copolymer
dc.rights.license | open | |
dc.contributor.author | MURTO, Petri | |
dc.contributor.author | GENENE, Zewdneh | |
dc.contributor.author | BENAVIDES, Cindy Montenegro | |
dc.contributor.author | XU, Xiaofeng | |
hal.structure.identifier | Laboratoire de Chimie des Polymères Organiques [LCPO] | |
hal.structure.identifier | Team 4 LCPO : Polymer Materials for Electronic, Energy, Information and Communication Technologies | |
dc.contributor.author | SHARMA, Anirudh | |
dc.contributor.author | PAN, Xun | |
dc.contributor.author | SCHMIDT, Oliver | |
dc.contributor.author | BRABEC, Christoph | |
hal.structure.identifier | Department of Mathematical Sciences | |
dc.contributor.author | ANDERSSON, Mats | |
dc.contributor.author | TEDDE, Sandro | |
dc.contributor.author | MAMMO, Wendimagegn | |
dc.contributor.author | WANG, Ergang | |
dc.date.accessioned | 2020 | |
dc.date.available | 2020 | |
dc.date.issued | 2018 | |
dc.identifier.issn | 2161-1653 | |
dc.identifier.uri | https://oskar-bordeaux.fr/handle/20.500.12278/20032 | |
dc.description.abstractEn | The synthesis of an acceptor polymer PIDT-2TPD, comprising indacenodithiophene (IDT) as theelectron-rich unit and an interconnected bithieno[3,4-c]-pyrrole-4,4′,6,6′-tetrone (2TPD) as the electron-deficientunit, and its application for all-polymer photodetectors isreported. The optical, electrochemical, charge transport, anddevice properties of a blend of poly(3-hexylthiophene) andPIDT-2TPD are studied. The blend shows strong complementaryabsorption and balanced electron and hole mobility,which are desired properties for a photoactive layer. Thedevice exhibits dark current density in the order of 10exp−5 mA/cm2, external quantum efficiency broadly above 30%, and nearly planar detectivity over the entire visible spectral range(maximum of 1.1 × 10exp12 Jones at 610 nm) under −5 V bias. These results indicate that PIDT-2TPD is a highly functional newtype of acceptor and further motivate the use of 2TPD as a building block for other n-type materials. | |
dc.language.iso | en | |
dc.publisher | Washington, D.C : American Chemical Society | |
dc.subject.en | Donor-acceptor copolymer | |
dc.subject.en | Photodetector | |
dc.title.en | High Performance All-Polymer Photodetector Comprising a Donor–Acceptor–Acceptor Structured Indacenodithiophene–Bithieno[3,4- c ]Pyrroletetrone Copolymer | |
dc.type | Article de revue | |
dc.identifier.doi | 10.1021/acsmacrolett.8b00009 | |
dc.subject.hal | Chimie/Polymères | |
dc.subject.hal | Sciences de l'ingénieur [physics]/Optique / photonique | |
bordeaux.journal | ACS Macro Letters | |
bordeaux.page | 395 - 400 | |
bordeaux.volume | 7 | |
bordeaux.hal.laboratories | Laboratoire de Chimie des Polymères Organiques (LCPO) - UMR 5629 | * |
bordeaux.issue | 4 | |
bordeaux.institution | Bordeaux INP | |
bordeaux.institution | Université de Bordeaux | |
bordeaux.peerReviewed | oui | |
hal.identifier | hal-01829896 | |
hal.version | 1 | |
hal.origin.link | https://hal.archives-ouvertes.fr//hal-01829896v1 | |
bordeaux.COinS | ctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=ACS%20Macro%20Letters&rft.date=2018&rft.volume=7&rft.issue=4&rft.spage=395%20-%20400&rft.epage=395%20-%20400&rft.eissn=2161-1653&rft.issn=2161-1653&rft.au=MURTO,%20Petri&GENENE,%20Zewdneh&BENAVIDES,%20Cindy%20Montenegro&XU,%20Xiaofeng&SHARMA,%20Anirudh&rft.genre=article |
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