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Critical Review on Sustainable Homogeneous Cellulose Modification: Why Renewability Is Not Enough

dc.rights.licenseopen
dc.contributor.authorONWUKAMIKE, Kelechukwu
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorGRELIER, Stéphane
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorGRAU, Etienne
IDREF: 187909261
hal.structure.identifierLaboratoire de Chimie des Polymères Organiques [LCPO]
hal.structure.identifierTeam 2 LCPO : Biopolymers & Bio-sourced Polymers
dc.contributor.authorCRAMAIL, Henri
hal.structure.identifierKarlsruhe Institute of Technology [KIT]
dc.contributor.authorMEIER, Michael
dc.date.accessioned2020
dc.date.available2020
dc.date.issued2018
dc.identifier.issn2168-0485
dc.identifier.urihttps://oskar-bordeaux.fr/handle/20.500.12278/19806
dc.description.abstractEnAs we passed the 20th anniversary of the publication of the 12 principles of green chemistry, the sustainable modification of cellulose, being the most abundant biobased polymer, is certainly worth considering. Many researchers work on an efficient valorization of this renewable resource due to its manifold and promising application possibilities, but very often the use of non-sustainable approaches (i.e., solvents, reactants and modification approaches) only addresses the renewability aspect of cellulose, while neglecting most or all of the other principles of green chemistry. In this review, we have employed the use of E-factors together with basic toxicity information to compare between various approaches for homogeneous cellulose modification. This approach, though simple and certainly not overarching, can provide a quick and useful first sustainability assessment. Therefore, in order to achieve a truly sustainable modification of cellulose, its renewability combined with mild and efficient reaction protocols is crucial in order to obtain sustainable materials that are capable of reducing the overall negative impact of today’s fossil-based polymeric materials.
dc.language.isoen
dc.publisherAmerican Chemical Society
dc.subject.enCellulose Homogeneous modification Sustainability E-factor
dc.title.enCritical Review on Sustainable Homogeneous Cellulose Modification: Why Renewability Is Not Enough
dc.typeArticle de revue
dc.identifier.doi10.1021/acssuschemeng.8b04990
dc.subject.halChimie/Polymères
dc.subject.halChimie/Matériaux
dc.subject.halChimie
dc.subject.halPhysique [physics]/Matière Condensée [cond-mat]/Science des matériaux [cond-mat.mtrl-sci]
dc.identifier.arxiv1911.07659
bordeaux.journalACS Sustainable Chemistry & Engineering
bordeaux.page1826-1840
bordeaux.volume7
bordeaux.hal.laboratoriesLaboratoire de Chimie des Polymères Organiques (LCPO) - UMR 5629*
bordeaux.issue2
bordeaux.institutionBordeaux INP
bordeaux.institutionUniversité de Bordeaux
bordeaux.peerReviewedoui
hal.identifierhal-02134692
hal.version1
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-02134692v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=ACS%20Sustainable%20Chemistry%20&%20Engineering&rft.date=2018&rft.volume=7&rft.issue=2&rft.spage=1826-1840&rft.epage=1826-1840&rft.eissn=2168-0485&rft.issn=2168-0485&rft.au=ONWUKAMIKE,%20Kelechukwu&GRELIER,%20St%C3%A9phane&GRAU,%20Etienne&CRAMAIL,%20Henri&MEIER,%20Michael&rft.genre=article


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