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Target and Nontarget Screening of PFAS in Biosolids, Composts, and Other Organic Waste Products for Land Application in France

hal.structure.identifierDépartement de chimie [UdeM-Montréal]
dc.contributor.authorMUNOZ, Gabriel
hal.structure.identifierEcologie fonctionnelle et écotoxicologie des agroécosystèmes [ECOSYS]
dc.contributor.authorMICHAUD, Aurélia Marcelline
hal.structure.identifierMcGill University = Université McGill [Montréal, Canada]
dc.contributor.authorLIU, Min
hal.structure.identifierDépartement de chimie [UdeM-Montréal]
dc.contributor.authorVO DUY, Sung
hal.structure.identifierService d'expérimentation agronomique et viticole [COLM AGRO VITI UE]
dc.contributor.authorMONTENACH, Denis
hal.structure.identifierEcologie fonctionnelle et écotoxicologie des agroécosystèmes [ECOSYS]
dc.contributor.authorRESSEGUIER, Camille
hal.structure.identifierLaboratoire Sols et Environnement [LSE]
dc.contributor.authorWATTEAU, Françoise
hal.structure.identifierInteractions Sol Plante Atmosphère [UMR ISPA]
dc.contributor.authorSAPPIN-DIDIER, Valérie
hal.structure.identifierRecyclage et risque [UPR Recyclage et risque]
dc.contributor.authorFEDER, Frédéric
hal.structure.identifierSol Agro et hydrosystème Spatialisation [SAS]
dc.contributor.authorMORVAN, Thierry
hal.structure.identifierEcologie fonctionnelle et écotoxicologie des agroécosystèmes [ECOSYS]
dc.contributor.authorHOUOT, Sabine
hal.structure.identifierCentre d'Expertise en Analyse Environnementale du Quebec
dc.contributor.authorDESROSIERS, Mélanie
hal.structure.identifierMcGill University = Université McGill [Montréal, Canada]
dc.contributor.authorLIU, Jinxia
hal.structure.identifierDépartement de chimie [UdeM-Montréal]
dc.contributor.authorSAUVÉ, Sébastien
dc.date.accessioned2024-04-08T11:48:59Z
dc.date.available2024-04-08T11:48:59Z
dc.date.issued2022
dc.identifier.issn0013-936X
dc.identifier.urihttps://oskar-bordeaux.fr/handle/20.500.12278/195320
dc.description.abstractEnZwitterionic, cationic, and anionic per- and polyfluoroalkyl substances (PFAS) are increasingly reported in terrestrial and aquatic environments, but their inputs to agricultural lands are not fully understood. Here, we characterized PFAS in 47 organic waste products (OWP) applied in agricultural fields of France, including historical and recent materials. Overall, 160 PFAS from 42 classes were detected from target screening and homologue-based nontarget screening. Target PFAS were low in agriculture-derived wastes such as pig slurry, poultry manure, or dairy cattle manure (median 46PFAS: 0.66 mug/kg dry matter). Higher PFAS levels were reported in urban and industrial wastes, paper mill sludge, sewage sludge, or residual household waste composts (median 46PFAS: 220 mug/kg). Historical municipal biosolids and composts (1976-1998) were dominated by perfluorooctanesulfonate (PFOS), N-ethyl perfluorooctanesulfonamido acetic acid (EtFOSAA), and cationic and zwitterionic electrochemical fluorination precursors to PFOS. Contemporaneous urban OWP (2009-2017) were rather dominated by zwitterionic fluorotelomers, which represented on average 55% of 160PFAS (max: 97%). The fluorotelomer sulfonamidopropyl betaines (X:2 FTSA-PrB, median: 110 mug/kg, max: 1300 mug/kg) were the emerging class with the highest occurrence and prevalence in contemporary urban OWP. They were also detected as early as 1985. The study informs for the first time that urban sludges and composts can be a significant repository of zwitterionic and cationic PFAS.
dc.description.sponsorshipANAEE-Services
dc.language.isoen
dc.publisherAmerican Chemical Society
dc.subject.ennontarget screening
dc.subject.enKendrick mass defect
dc.subject.encationic and zwitterionic PFAS
dc.subject.enfluorotelomers
dc.subject.enmunicipal biosolids
dc.subject.encomposts
dc.subject.enagricultural wastes
dc.subject.entemporal shift
dc.title.enTarget and Nontarget Screening of PFAS in Biosolids, Composts, and Other Organic Waste Products for Land Application in France
dc.typeArticle de revue
dc.identifier.doi10.1021/acs.est.1c03697
dc.subject.halSciences de l'environnement
bordeaux.journalEnvironmental Science and Technology
bordeaux.page6056-6068
bordeaux.volume56
bordeaux.hal.laboratoriesInteractions Soil Plant Atmosphere (ISPA) - UMR 1391*
bordeaux.issue10
bordeaux.institutionBordeaux Sciences Agro
bordeaux.institutionINRAE
bordeaux.peerReviewedoui
hal.identifierhal-03561958
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-03561958v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Environmental%20Science%20and%20Technology&rft.date=2022&rft.volume=56&rft.issue=10&rft.spage=6056-6068&rft.epage=6056-6068&rft.eissn=0013-936X&rft.issn=0013-936X&rft.au=MUNOZ,%20Gabriel&MICHAUD,%20Aur%C3%A9lia%20Marcelline&LIU,%20Min&VO%20DUY,%20Sung&MONTENACH,%20Denis&rft.genre=article


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