Chiral discrimination in helicity-preserving Fabry-Pérot cavities
| hal.structure.identifier | Laboratoire Ondes et Matière d'Aquitaine [LOMA] | |
| dc.contributor.author | MAURO, L. | |
| hal.structure.identifier | Universidad Autónoma de Madrid [UAM] | |
| dc.contributor.author | FREGONI, J. | |
| hal.structure.identifier | Universidad Autónoma de Madrid [UAM] | |
| dc.contributor.author | FEIST, J. | |
| hal.structure.identifier | Laboratoire Ondes et Matière d'Aquitaine [LOMA] | |
| dc.contributor.author | AVRILLER, Rémi | |
| dc.date.issued | 2023-02 | |
| dc.identifier.issn | 2469-9926 | |
| dc.description.abstractEn | We theoretically study circular dichroism of chiral molecules embedded inside a helicity-preserving Fabry-Pérot cavity. We find an increase of the intrinsic chiroptical response of the molecules by 2 orders of magnitude and report the first clear signature of chiral cavity polaritons upon entering the regime of strong light-matter coupling. We study a cavity design based on two dielectric photonic crystal mirrors acting, in a narrow frequency range, as efficient polarization cross-converters in transmission for one polarization and almost perfect reflectors for the other polarization. We show that a Pasteur medium hosted inside such a cavity can couple efficiently to both the outside of the cavity and to the helicity-preserving mode, inheriting an enhanced chiral character. We expect such a device to be useful in the future to design ultrasensitive chiral sensors for optics andstereochemistry. | |
| dc.description.sponsorship | Réactions Chimiques, Transfert de Charges et d'Energie en Cavité Electromagnétique - ANR-18-CE30-0006 | |
| dc.language.iso | en | |
| dc.publisher | American Physical Society | |
| dc.subject.en | Chirality | |
| dc.subject.en | Polaritons | |
| dc.subject.en | Polarization of light | |
| dc.subject.en | Cavity methods | |
| dc.title.en | Chiral discrimination in helicity-preserving Fabry-Pérot cavities | |
| dc.type | Article de revue | |
| dc.identifier.doi | 10.1103/PhysRevA.107.L021501 | |
| dc.subject.hal | Physique [physics]/Matière Condensée [cond-mat] | |
| dc.subject.hal | Physique [physics]/Physique [physics]/Optique [physics.optics] | |
| dc.identifier.arxiv | 2209.00402 | |
| bordeaux.journal | Physical Review A | |
| bordeaux.page | L021501 | |
| bordeaux.volume | 107 | |
| bordeaux.issue | 2 | |
| bordeaux.peerReviewed | oui | |
| hal.identifier | hal-04000433 | |
| hal.version | 1 | |
| hal.popular | non | |
| hal.audience | Internationale | |
| hal.origin.link | https://hal.archives-ouvertes.fr//hal-04000433v1 | |
| bordeaux.COinS | ctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Physical%20Review%20A&rft.date=2023-02&rft.volume=107&rft.issue=2&rft.spage=L021501&rft.epage=L021501&rft.eissn=2469-9926&rft.issn=2469-9926&rft.au=MAURO,%20L.&FREGONI,%20J.&FEIST,%20J.&AVRILLER,%20R%C3%A9mi&rft.genre=article |
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