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Imperfect narrow escape problem

hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
dc.contributor.authorGUÉRIN, Thomas
hal.structure.identifierLaboratoire de Physique Théorique de la Matière Condensée [LPTMC]
dc.contributor.authorDOLGUSHEV, M.
hal.structure.identifierLaboratoire de Physique Théorique de la Matière Condensée [LPTMC]
dc.contributor.authorBÉNICHOU, O.
hal.structure.identifierLaboratoire Jean Perrin [LJP]
hal.structure.identifierLaboratoire de Physique Théorique de la Matière Condensée [LPTMC]
dc.contributor.authorVOITURIEZ, R.
dc.date.issued2023
dc.identifier.issn2470-0045
dc.description.abstractEnWe consider the kinetics of the imperfect narrow escape problem, i.e. the time it takes for a particle diffusing in a confined medium of generic shape to reach and to be adsorbed by a small, imperfectly reactive patch embedded in the boundary of the domain, in two or three dimensions. Imperfect reactivity is modeled by an intrinsic surface reactivity κ of the patch, giving rise to Robin boundary conditions. We present a formalism to calculate the exact asymptotics of the mean reaction time in the limit of large volume of the confining domain. We obtain exact explicit results in the two limits of large and small reactivities of the reactive patch, and a semi-analytical expression in the general case. Our approach reveals an anomalous scaling of the mean reaction time as the inverse square root of the reactivity in the large reactivity limit, valid for an initial position near the extremity of the reactive patch. We compare our exact results with those obtained within the "constant flux approximation"; we show that this approximation turns out to give exactly the next-to-leading order term of the small reactivity limit, and provides a good approximation of the reaction time far from the reactive patch for all reactivities, but not in the vicinity of the boundary of the reactive patch due to the above mentioned anomalous scaling. These results thus provide a general framework to quantify the mean reaction times for the imperfect narrow escape problem.
dc.description.sponsorshipPremières rencontres en environnement complexe - ANR-21-CE30-0020
dc.language.isoen
dc.publisherAmerican Physical Society (APS)
dc.title.enImperfect narrow escape problem
dc.typeArticle de revue
dc.identifier.doi10.1103/PhysRevE.107.034134
dc.subject.halPhysique [physics]/Matière Condensée [cond-mat]/Mécanique statistique [cond-mat.stat-mech]
bordeaux.journalPhysical Review E
bordeaux.page034134
bordeaux.volume107
bordeaux.issue3
bordeaux.peerReviewedoui
hal.identifierhal-04093907
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-04093907v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Physical%20Review%20E&rft.date=2023&rft.volume=107&rft.issue=3&rft.spage=034134&rft.epage=034134&rft.eissn=2470-0045&rft.issn=2470-0045&rft.au=GU%C3%89RIN,%20Thomas&DOLGUSHEV,%20M.&B%C3%89NICHOU,%20O.&VOITURIEZ,%20R.&rft.genre=article


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