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Improved electrochemical performance for high voltage spinel LiNi0.5Mn1.5O4 modified by supercritical fluid chemical deposition

hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierTechnocentre, Renault SAS
dc.contributor.authorCOURBARON, Gwenaëlle
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
dc.contributor.authorPETIT, Emmanuel
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierAdvanced Lithium Energy Storage Systems - ALISTORE-ERI [ALISTORE-ERI]
hal.structure.identifierCIC ENERGIGUNE - Parque Tecnol Alava
dc.contributor.authorSERRANO-SEVILLANO, Jon
hal.structure.identifierPlateforme Aquitaine de Caractérisation des Matériaux [PLACAMAT]
dc.contributor.authorLABRUGÈRE-SARROSTE, Christine
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
hal.structure.identifierAdvanced Lithium Energy Storage Systems - ALISTORE-ERI [ALISTORE-ERI]
dc.contributor.authorOLCHOWKA, Jacob
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
hal.structure.identifierAdvanced Lithium Energy Storage Systems - ALISTORE-ERI [ALISTORE-ERI]
dc.contributor.authorCARLIER, Dany
hal.structure.identifierTechnocentre, Renault SAS
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
hal.structure.identifierAdvanced Lithium Energy Storage Systems - ALISTORE-ERI [ALISTORE-ERI]
dc.contributor.authorDELPUECH, Nathalie
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
dc.contributor.authorAYMONIER, Cyril
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierRéseau sur le stockage électrochimique de l'énergie [RS2E]
hal.structure.identifierAdvanced Lithium Energy Storage Systems - ALISTORE-ERI [ALISTORE-ERI]
dc.contributor.authorCROGUENNEC, Laurence
dc.date.issued2023-01-18
dc.identifier.issn1944-8244
dc.description.abstractEnAmong candidates at the positive electrode of the next generation of Li-ion technology and even beyond post Li-ion technology as all-solid-state batteries, spinel LiNi0.5Mn1.5O4 (LNMO) is one of the favorites. Nevertheless, before its integration into commercial systems, challenges still remain to be tackled, especially the stabilization of interfaces with the electrolyte (liquid or solid) at high voltage. In this work, a simple, fast, and cheap process is used to prepare a homogeneous coating of Al2O3 type to modify the surface of the spinel LNMO: the supercritical fluid chemical deposition (SFCD) route. This process is, to the best of our knowledge, used for the first time in the battery field. Significantly improved performance was demonstrated vs those of bare LNMO, especially at high rates and for highly loaded electrodes.
dc.description.sponsorshipLaboratory of excellency for electrochemical energy storage
dc.language.isoen
dc.publisherWashington, D.C. : American Chemical Society
dc.subject.enLithium-ion batteries
dc.subject.enSurface modification
dc.subject.enHigh-voltage positive electrode material
dc.subject.enSpinel oxide LiNi0.5Mn1.5O4
dc.subject.enSupercritical fluid chemical deposition
dc.title.enImproved electrochemical performance for high voltage spinel LiNi0.5Mn1.5O4 modified by supercritical fluid chemical deposition
dc.typeArticle de revue
dc.identifier.doi10.1021/acsami.2c14777
dc.subject.halChimie/Matériaux
bordeaux.journalACS Applied Materials & Interfaces
bordeaux.page2812-2824
bordeaux.volume15
bordeaux.issue2
bordeaux.peerReviewedoui
hal.identifierhal-03947373
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-03947373v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=ACS%20Applied%20Materials%20&%20Interfaces&rft.date=2023-01-18&rft.volume=15&rft.issue=2&rft.spage=2812-2824&rft.epage=2812-2824&rft.eissn=1944-8244&rft.issn=1944-8244&rft.au=COURBARON,%20Gwena%C3%ABlle&PETIT,%20Emmanuel&SERRANO-SEVILLANO,%20Jon&LABRUG%C3%88RE-SARROSTE,%20Christine&OLCHOWKA,%20Jacob&rft.genre=article


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