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hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorTAMARAT, P.
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorJELEZKO, F.
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorBRUNEL, C.
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorMAALI, A.
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorLOUNIS, B.
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorORRIT, M.
dc.date.created1998-10-29
dc.date.issued1999-07
dc.identifier.issn0301-0104
dc.description.abstractEnWe review several recent non-linear optical experiments done with single molecules in molecular crystals at low temperatures. We summarize pump–probe experiments showing light-shift, hyper-Raman and subharmonic resonances, electro-optical effects in which laser and RF frequencies are mixed by a single molecule, and the proposed use of a molecule as a triggered single-photon emitter. The comparison of experimental results to a simple two-level model with optical Bloch equations shows that single molecules are accurately described as electronic two-level systems and that they are very convenient testbenches for many investigations in non-linear and quantum optics.
dc.language.isoen
dc.publisherElsevier
dc.title.enNon-linear optical response of single molecules
dc.typeArticle de revue
dc.identifier.doi10.1016/S0301-0104(99)00024-5
dc.subject.halPhysique [physics]
bordeaux.journalChemical Physics
bordeaux.page121-132
bordeaux.volume245
bordeaux.issue1-3
bordeaux.peerReviewedoui
hal.identifierhal-01550385
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-01550385v1
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