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Non-linear optical response of single molecules
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | TAMARAT, P. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | JELEZKO, F. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | BRUNEL, C. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | MAALI, A. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | LOUNIS, B. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | ORRIT, M. | |
dc.date.created | 1998-10-29 | |
dc.date.issued | 1999-07 | |
dc.identifier.issn | 0301-0104 | |
dc.description.abstractEn | We review several recent non-linear optical experiments done with single molecules in molecular crystals at low temperatures. We summarize pump–probe experiments showing light-shift, hyper-Raman and subharmonic resonances, electro-optical effects in which laser and RF frequencies are mixed by a single molecule, and the proposed use of a molecule as a triggered single-photon emitter. The comparison of experimental results to a simple two-level model with optical Bloch equations shows that single molecules are accurately described as electronic two-level systems and that they are very convenient testbenches for many investigations in non-linear and quantum optics. | |
dc.language.iso | en | |
dc.publisher | Elsevier | |
dc.title.en | Non-linear optical response of single molecules | |
dc.type | Article de revue | |
dc.identifier.doi | 10.1016/S0301-0104(99)00024-5 | |
dc.subject.hal | Physique [physics] | |
bordeaux.journal | Chemical Physics | |
bordeaux.page | 121-132 | |
bordeaux.volume | 245 | |
bordeaux.issue | 1-3 | |
bordeaux.peerReviewed | oui | |
hal.identifier | hal-01550385 | |
hal.version | 1 | |
hal.popular | non | |
hal.audience | Internationale | |
hal.origin.link | https://hal.archives-ouvertes.fr//hal-01550385v1 | |
bordeaux.COinS | ctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Chemical%20Physics&rft.date=1999-07&rft.volume=245&rft.issue=1-3&rft.spage=121-132&rft.epage=121-132&rft.eissn=0301-0104&rft.issn=0301-0104&rft.au=TAMARAT,%20P.&JELEZKO,%20F.&BRUNEL,%20C.&MAALI,%20A.&LOUNIS,%20B.&rft.genre=article |
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