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hal.structure.identifierDepartment of Physics and Astronomy [Hamilton, ON]
dc.contributor.authorSCHULMAN, Rafael
hal.structure.identifierLaboratoire de Physico-Chimie Théorique [LPCT]
dc.contributor.authorTREJO, Miguel
hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
hal.structure.identifierGlobal Station for Soft Matter, Global Institution for Collaborative Research and Education [Hokkaido]
dc.contributor.authorSALEZ, Thomas
hal.structure.identifierLaboratoire de Physico-Chimie Théorique [LPCT]
dc.contributor.authorRAPHAËL, Elie
hal.structure.identifierLaboratoire de Physico-Chimie Théorique [LPCT]
hal.structure.identifierDepartment of Physics and Astronomy [Hamilton, ON]
dc.contributor.authorDALNOKI-VERESS, Kari
dc.date.issued2018
dc.identifier.issn2041-1723
dc.description.abstractEnSurface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, since their surface energies change with strain. Crystalline materials are known to have strain-dependent surface energies, but in amorphous materials, such as polymeric glasses and elastomers, the strain dependence is debated due to a dearth of direct measurements. Here, we utilize contact angle measurements on strained glassy and elas-tomeric solids to address this matter. We show conclusively that interfaces involving poly-meric glasses exhibit strain-dependent surface energies, and give strong evidence for the absence of such a dependence for incompressible elastomers. The results provide fundamental insight into our understanding of the interfaces of amorphous solids and their interaction with contacting liquids.
dc.language.isoen
dc.publisherNature Publishing Group
dc.rights.urihttp://creativecommons.org/licenses/by/
dc.title.enSurface energy of strained amorphous solids
dc.typeArticle de revue
dc.identifier.doi10.1038/s41467-018-03346-1
dc.subject.halPhysique [physics]/Matière Condensée [cond-mat]/Science des matériaux [cond-mat.mtrl-sci]
bordeaux.journalNature Communications
bordeaux.page982
bordeaux.volume9
bordeaux.issue1
bordeaux.peerReviewedoui
hal.identifierhal-01804460
hal.version1
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-01804460v1
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