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Effects of confinement on the electron and lattice dynamics in metal nanoparticles
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | LERMÉ, J. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | CELEP, G. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | BROYER, M. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | COTTANCIN, E. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | PELLARIN, M. | |
hal.structure.identifier | Centre d'élaboration de matériaux et d'études structurales [CEMES] | |
dc.contributor.author | ARBOUET, Arnaud | |
dc.contributor.author | CHRISTOFILOS, D. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | GUILLON, C. | |
hal.structure.identifier | Centre de physique moléculaire optique et hertzienne [CPMOH] | |
dc.contributor.author | LANGOT, P. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | DEL FATTI, N. | |
hal.structure.identifier | Laboratoire de Spectrométrie Ionique et Moléculaire [LASIM] | |
dc.contributor.author | VALLÉE, F. | |
dc.date.created | 2005-07-13 | |
dc.date.issued | 2005-07-13 | |
dc.identifier.issn | 1434-6060 | |
dc.description.abstractEn | Effects of confinement on the electron-electron (e-e) and electron-phonon (e-ph) thermalization dynamics in noble metal clusters are calculated using simple approaches. The model predictions are compared with femtosecond pump-probe measurements which display an acceleration of the e-e and e-ph relaxation dynamics. The size-effects on the e-e relaxation dynamics are consistent with a model involving the surface-induced reduction of the screening efficiency of the Coulomb e-e interaction. With regard to the e-ph relaxation dynamics, this model yields too large time constants, pointing out deficiencies of the standard modelling of the e-ph energy exchanges in bulk metals. Analysis of these deficiencies shows that the bare e-ion interaction has to be involved in the transition matrix element describing the non-adiabatic e-ph energy exchanges. | |
dc.language.iso | en | |
dc.publisher | EDP Sciences | |
dc.title.en | Effects of confinement on the electron and lattice dynamics in metal nanoparticles | |
dc.type | Article de revue | |
dc.identifier.doi | 10.1140/epjd/e2005-00107-8 | |
bordeaux.journal | The European Physical Journal D : Atomic, molecular, optical and plasma physics | |
bordeaux.page | 199 | |
bordeaux.volume | 34 | |
bordeaux.peerReviewed | oui | |
hal.identifier | hal-00342467 | |
hal.version | 1 | |
hal.popular | non | |
hal.audience | Internationale | |
hal.origin.link | https://hal.archives-ouvertes.fr//hal-00342467v1 | |
bordeaux.COinS | ctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=The%20European%20Physical%20Journal%20D%20:%20Atomic,%20molecular,%20optical%20and%20plasma%20physics&rft.date=2005-07-13&rft.volume=34&rft.spage=199&rft.epage=199&rft.eissn=1434-6060&rft.issn=1434-6060&rft.au=LERM%C3%89,%20J.&CELEP,%20G.&BROYER,%20M.&COTTANCIN,%20E.&PELLARIN,%20M.&rft.genre=article |
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