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Development and Experimental Demonstration of Negative First-Order Quasi-Phase Matching in a periodically-poled Rb-doped KTiOPO4 crystal

hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierCentre d'Etudes Lasers Intenses et Applications [CELIA]
dc.contributor.authorPETIT, Yannick
hal.structure.identifierOptique et Matériaux [NEEL - OPTIMA]
dc.contributor.authorPENA, Alexandra
hal.structure.identifierOptique et Matériaux [NEEL - OPTIMA]
dc.contributor.authorSEGONDS, Patricia
hal.structure.identifierCristaux massifs [NEEL - CrisMass]
dc.contributor.authorDEBRAY, Jérôme
hal.structure.identifierLaboratoire de l'intégration, du matériau au système [IMS]
dc.contributor.authorJOLY, Simon
hal.structure.identifierKTH Royal Institute of Technology [Stockholm] [KTH]
dc.contributor.authorZUKAUSKAS, Andrius
hal.structure.identifierKTH Royal Institute of Technology [Stockholm] [KTH]
dc.contributor.authorLAURELL, Fredrik
hal.structure.identifierKTH Royal Institute of Technology [Stockholm] [KTH]
dc.contributor.authorPASISKEVICIUS, Valdas
hal.structure.identifierKTH Royal Institute of Technology [Stockholm] [KTH]
dc.contributor.authorCANALIAS, Carlota
hal.structure.identifierOptique et Matériaux [NEEL - OPTIMA]
dc.contributor.authorBOULANGER, Benoit
dc.date.issued2020
dc.identifier.issn0146-9592
dc.description.abstractEnWe worked on a new scheme of Quasi-Phase-Matching (QPM) based on the negative first-order of the spatial modulation of the sign of the second-order nonlinearity. Applying this scheme in the case of Angular-Quasi-Phase-Matching (AQPM) in a biaxial crystal reveals new directions of propagation for efficient parametric frequency conversion as well as "giant" spectral acceptances. The experimental validation is performed in a periodically-poled Rubidium-doped KTiOPO4 biaxial crystal. This new approach naturally extends to other periodically-poled uniaxial crystals such as periodically-poled LiNbO3. Phase-matching is the privileged way to optimize the performance of nonlinear optical frequency conversion. Usually, it can be obtained by using the birefringence of anisotropic crystals, which corresponds to birefringence phase-matching (BPM) [1,2]. However, BPM conditions are strongly limited by the refractive indices of the material and they usually forbid the exploitation of the highest coefficient of the second-order electric susceptibility tensor. To overcome this limitation, quasi-phase matching (QPM) is a powerful alternative. It is based on a periodical modulation of the sign of the second-order optical nonlinear coefficient of anisotropic or isotropic non-centrosymmetric crystals [3,4]. We propose here the development and the experimental validation of a new scheme of QPM that allows us to enlarge the spectral range of phase-matched generation and to get access to giant spectral acceptances. For that purpose, we studied Second-Harmonic Generation (SHG) in the ferroelectric periodically-poled Rubidium-doped KTiOPO4 crystal (PPRKTP) [5]. The key parameter of QPM is the periodicity Λ of the spatial modulation of the second-order nonlinearity along the direction of propagation of three interacting waves such as their wavelengths fulfil: 1/λ ! − 1/λ " − 1/λ # = 0. Actually, the goal is to compensate the #% ' , is the grating vector oriented along the propagation direction, and m is the order of the Fourier series. Usually, m is chosen as a positive integer (m ≥ 1), as it is the case for instance while targeting the largest nonlinear coefficient χ !! (#). It is shown in Fig. 1 (left) in the optimal case, i.e. for the lowest QPM positive order m = 1. This is the classical scheme of QPM that we called QPM-A. However, it is also possible to consider propagation directions where m ≤-1. This configuration has been previously theoretically considered, but without any phenomenological interpretation or experimental verification [6]. We called here this new scheme QPM-B. As for the case of positive orders, the lowest QPM-B order (namely m =-1) shown in Fig. 1 (right) leads to the best efficiency compared to higher
dc.language.isoen
dc.publisherOptical Society of America - OSA Publishing
dc.title.enDevelopment and Experimental Demonstration of Negative First-Order Quasi-Phase Matching in a periodically-poled Rb-doped KTiOPO4 crystal
dc.typeArticle de revue
dc.identifier.doi10.1364/OL.408839
dc.subject.halChimie/Matériaux
bordeaux.journalOptics Letters
bordeaux.page6026-6029
bordeaux.volume45
bordeaux.issue21
bordeaux.peerReviewedoui
hal.identifierhal-02953325
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-02953325v1
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