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Three-dimensional high spatial localization of efficient resonant energy transfer from laser-assisted precipitated silver clusters to trivalent Europium ions

hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierCentre d'Etudes Lasers Intenses et Applications [CELIA]
dc.contributor.authorPETIT, Yannick
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
hal.structure.identifierUniversidade de São Paulo = University of São Paulo [USP]
dc.contributor.authorGALLEANI, Gustavo
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorRAFFY, Guillaume
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorDESMOULIN, Jean-Charles
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorJUBERA, Veronique
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorDEL GUERZO, André
hal.structure.identifierUniversidade de São Paulo = University of São Paulo [USP]
dc.contributor.authorSTUCCHI DE CAMARGO, Andrea Simone
hal.structure.identifierCentre d'Etudes Lasers Intenses et Applications [CELIA]
dc.contributor.authorCANIONI, Lionel
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorCARDINAL, Thierry
dc.date.issued2021
dc.identifier.issn2073-4352
dc.description.abstractEnWe report on the 3D precipitation, using a direct laser writing approach, of highly fluorescent silver clusters in a Eu 3+-doped silvercontaining zinc phosphate glass. Micro-spectroscopy of fluorescence emission shows the ability to continuously adjust the local trichromatic coordinates in the CIE chromaticity diagram between red and white colors, thanks to the laser-deposited dose and resulting tunable combination of emissions from Eu 3+ and silver clusters. Moreover, CW and time-resolved FAST-FLIM spectroscopies showed a significant enhancement of the fluorescence emission of Eu 3+ ions while being co-located with UV-excited laser-inscribed silver clusters. These results demonstrate the ability to perform efficient resonant non-radiative energy transfer from excited silver clusters to Eu 3+ , allowing such energy transfer to be highly localized on demand thanks to laser inscription. Such results open the route to 3D printing of the rare earth ions emission in glass.
dc.description.sponsorshipArchitectures photoniques intégrées inscrites par laser femtoseconde pour étalonnage en microscopie de fluorescence dans l'infrarouge - ANR-19-CE08-0021
dc.language.isoen
dc.publisherMDPI
dc.subject.ensilver clusters
dc.subject.enrare earth ions
dc.subject.enfemtosecond laser inscription
dc.subject.enFLIM spectroscopy
dc.subject.enresonant transfers
dc.subject.enDexter process
dc.subject.enFRET process
dc.subject.enCIE chomaticity diagram
dc.title.enThree-dimensional high spatial localization of efficient resonant energy transfer from laser-assisted precipitated silver clusters to trivalent Europium ions
dc.typeArticle de revue
dc.identifier.doi10.3390/cryst11020148
dc.subject.halChimie/Matériaux
dc.subject.halChimie/Chimie inorganique
bordeaux.journalCrystals
bordeaux.page148
bordeaux.volume11
bordeaux.issue2
bordeaux.peerReviewedoui
hal.identifierhal-03130650
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-03130650v1
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