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Evolution of the linear and nonlinear optical properties of femtosecond laser exposed fused silica

hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
hal.structure.identifierThe College of Optics and Photonics [Orlando] [CREOL]
dc.contributor.authorROYON, Arnaud
hal.structure.identifierThe College of Optics and Photonics [Orlando] [CREOL]
hal.structure.identifierLockheed Martin Corporation
dc.contributor.authorRIVERO-BALEINE, Clara
hal.structure.identifierThe College of Optics and Photonics [Orlando] [CREOL]
hal.structure.identifierRaman Division
dc.contributor.authorZOUBIR, Arnaud
hal.structure.identifierCentre de physique moléculaire optique et hertzienne [CPMOH]
dc.contributor.authorCANIONI, Lionel
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorCOUZI, Michel
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorCARDINAL, Thierry
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorFARGIN, Evelyne
hal.structure.identifierThe College of Optics and Photonics [Orlando] [CREOL]
dc.contributor.authorRICHARDSON, Martin
hal.structure.identifierSchool of Materials Science and Engineering
dc.contributor.authorRICHARDSON, Kathleen
dc.date.issued2009
dc.identifier.issn0740-3224
dc.description.abstractEnThree fused silica samples possessing different impurity levels and exposed to a near infrared femtosecond laser are investigated. The laser-induced defects are identified from absorption, luminescence, and Raman spectroscopy. Their linear and nonlinear optical properties are measured from Kramers-Krönig calculations and third-harmonic generation microscopy experiments. No conclusive correlation between the change in the optical properties, the initial impurity levels, and the photoinduced structures could be established based on the results obtained in this study. In addition, several hypotheses (densification and color center formation) have been rejected to explain why the linear and nonlinear optical properties of the photoinduced structures follow a contradicting evolution. This phenomenon is attributed to an experimental artifact on the measurement of the third-order susceptibility due to scattering of the photoinduced structures.
dc.language.isoen
dc.publisherOptical Society of America
dc.title.enEvolution of the linear and nonlinear optical properties of femtosecond laser exposed fused silica
dc.typeArticle de revue
dc.identifier.doi10.1364/JOSAB.26.002077
dc.subject.halChimie/Matériaux
bordeaux.journalJournal of the Optical Society of America B
bordeaux.page2077-2083
bordeaux.volume26
bordeaux.issue11
bordeaux.peerReviewedoui
hal.identifierhal-00442688
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-00442688v1
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