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Synthesis and multiscale evaluation of LiNbO3 - Containing silicate glass-ceramics with efficient isotropic SHG response

hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorVIGOUROUX, Hélène
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorFARGIN, Evelyne
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorGOMEZ, Sonia
hal.structure.identifierCentre d'études scientifiques et techniques d'Aquitaine [CESTA]
dc.contributor.authorLE GARREC, Bruno
hal.structure.identifierTheoretical and Physical Chemistry Institute
dc.contributor.authorMOUNTRICHAS, Grigoris
hal.structure.identifierTheoretical and Physical Chemistry Institute
dc.contributor.authorKAMITSOS, Efstratios I.
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorADAMIETZ, Frédéric
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorDUSSAUZE, Marc
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorRODRIGUEZ, Vincent
dc.date.issued2012
dc.identifier.issn1616-301X
dc.description.abstractEnA study of bulk second harmonic generation (SHG) response of lithium niobium silicate glass-ceramics is presented. The observed macroscopic SHG signals have an isotropic 3D nature. To interpret this particular nonlinear optical response, a multiscale approach is used in which clear correlations between structure and optical response are characterized from the sub-micrometer to the millimeter scale. In particular, it is inferred that the radial distribution of the LiNbO3 crystallites in spherulite domains is at the origin of the isotropic bulk second order optical property. It is suggested that spherulitic crystallization in glass-ceramic is a challenging method to elaborate isotropic nonlinear optical properties in inorganic materials.
dc.language.isoen
dc.publisherWiley
dc.subject.enGlass-ceramic
dc.subject.enSpherulite crystallization
dc.subject.enNonlinear optical properties
dc.subject.enRaman spectroscopy
dc.subject.enSecond harmonic generation
dc.title.enSynthesis and multiscale evaluation of LiNbO3 - Containing silicate glass-ceramics with efficient isotropic SHG response
dc.typeArticle de revue
dc.identifier.doi10.1002/adfm.201200651
dc.subject.halChimie/Matériaux
bordeaux.journalAdvanced Functional Materials
bordeaux.page3985-3993
bordeaux.volume22
bordeaux.issue19
bordeaux.peerReviewedoui
hal.identifierhal-00751543
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-00751543v1
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