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Development of methods for the preparation of radiopure $^{82}$Se sources for the SuperNEMO neutrinoless double-beta decay experiment

dc.contributor.authorRAKHIMOV, Alimardon V.
dc.contributor.authorBARABASH, A.S.
dc.contributor.authorBASHARINA-FRESHVILLE, A.
dc.contributor.authorBLOT, S.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorBONGRAND, M.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorBOURGEOIS, Ch.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorBRETON, D.
dc.contributor.authorBREIER, R.
dc.contributor.authorBIRDSALL, E.
dc.contributor.authorBRUDANIN, V.B.
dc.contributor.authorBUREŠOVA, H.
hal.structure.identifierCentre de Physique des Particules de Marseille [CPPM]
dc.contributor.authorBUSTO, J.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorCALVEZ, S.
dc.contributor.authorCASCELLA, M.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorCERNA, C.
dc.contributor.authorCESAR, J.P.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorCHAUVEAU, E.
dc.contributor.authorCHOPRA, A.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorCLAVERIE, G.
dc.contributor.authorCAPUA, S.De
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorDELALEE, F.
hal.structure.identifierLaboratoire d'Annecy de Physique des Particules [LAPP]
dc.contributor.authorDUCHESNEAU, D.
dc.contributor.authorEGOROV, V.G.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorEURIN, G.
dc.contributor.authorEVANS, J.J.
dc.contributor.authorFAJT, L.
dc.contributor.authorFILOSOFOV, D.V.
dc.contributor.authorFLACK, R.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorGARRIDO, X.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorGOMEZ, H.
hal.structure.identifierLaboratoire de physique corpusculaire de Caen [LPCC]
dc.contributor.authorGUILLON, B.
dc.contributor.authorGUZOWSKI, P.
dc.contributor.authorHODÁK, R.
dc.contributor.authorHOLÝ, K.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorHUBER, A.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorHUGON, C.
hal.structure.identifierLaboratoire d'Annecy de Physique des Particules [LAPP]
dc.contributor.authorJEREMIE, A.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorJULLIAN, S.
dc.contributor.authorKARAIVANOV, D.V.
dc.contributor.authorKAUER, M.
dc.contributor.authorKLIMENKO, A.A.
dc.contributor.authorKOCHETOV, O.I.
dc.contributor.authorKONOVALOV, S.I.
dc.contributor.authorKOVALENKO, V.
dc.contributor.authorLANG, K.
hal.structure.identifierLaboratoire de physique corpusculaire de Caen [LPCC]
dc.contributor.authorLEMIÈRE, Y.
hal.structure.identifierLaboratoire d'Annecy de Physique des Particules [LAPP]
dc.contributor.authorNOBLET, T.Le
dc.contributor.authorLIPTAK, Z.
dc.contributor.authorLIU, X.R.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorLOAIZA, P.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorLUTTER, G.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorMAALMI, J.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorMACKO, M.
dc.contributor.authorMAMEDOV, F.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorMARQUET, C.
hal.structure.identifierLaboratoire de physique corpusculaire de Caen [LPCC]
dc.contributor.authorMAUGER, F.
hal.structure.identifierLaboratoire d'Annecy de Physique des Particules [LAPP]
dc.contributor.authorMINOTTI, A.
dc.contributor.authorMIRSAGATOVA, A.A.
dc.contributor.authorMIRZAYEV, N.A.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorMOREAU, I.
dc.contributor.authorMORGAN, B.
dc.contributor.authorMOTT, J.
dc.contributor.authorNEMCHENOK, I.B.
dc.contributor.authorNOMACHI, M.
dc.contributor.authorNOVA, F.
dc.contributor.authorOHSUMI, H.
hal.structure.identifierLaboratoire de physique corpusculaire de Caen [LPCC]
dc.contributor.authorOLIVIERO, G.
dc.contributor.authorPAHLKA, R.B.
dc.contributor.authorPATER, J.R.
dc.contributor.authorPALUŠOVÁ, V.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorPERROT, F.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorPIQUEMAL, F.
dc.contributor.authorPOVINEC, P.
dc.contributor.authorPRIDAL, P.
dc.contributor.authorRAMACHERS, Y.A.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorREBII, A.
hal.structure.identifierLaboratoire d'Annecy de Physique des Particules [LAPP]
dc.contributor.authorREMOTO, A.
dc.contributor.authorRICHARDS, B.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorRICOL, J.S.
dc.contributor.authorRUKHADZE, E.
dc.contributor.authorRUKHADZE, N.I.
dc.contributor.authorSAAKYAN, R.
dc.contributor.authorSADIKOV, I.I.
dc.contributor.authorSALAZAR, R.
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorSARAZIN, X.
dc.contributor.authorSEDGBEER, J.
dc.contributor.authorSHITOV, Yu. A.
dc.contributor.authorŠIMKOVIC, F.
hal.structure.identifierInstitut universitaire de France [IUF]
hal.structure.identifierLaboratoire de l'Accélérateur Linéaire [LAL]
dc.contributor.authorSIMARD, L.
dc.contributor.authorSMETANA, A.
dc.contributor.authorSMOLEK, K.
dc.contributor.authorSMOLNIKOV, A.A.
dc.contributor.authorSNOW, S.
dc.contributor.authorSÖLDNER-REMBOLD, S.
hal.structure.identifierCentre d'Etudes Nucléaires de Bordeaux Gradignan [CENBG]
dc.contributor.authorSOULÉ, B.
dc.contributor.authorŠPAVOROVA, M.
dc.contributor.authorŠTEKL, I.
dc.contributor.authorTASHIMOVA, F.A.
dc.contributor.authorTHOMAS, J.
dc.contributor.authorTIMKIN, V.
dc.contributor.authorTORRE, S.
dc.contributor.authorTRETYAK, Vl. I.
dc.contributor.authorTRETYAK, V.I.
dc.contributor.authorUMATOV, V.I.
dc.contributor.authorVILELA, C.
dc.contributor.authorVOROBEL, V.
hal.structure.identifierLaboratoire de Physique Subatomique et de Cosmologie [LPSC]
dc.contributor.authorWAROT, G.
dc.contributor.authorWATERS, D.
hal.structure.identifierLaboratoire de Physique Subatomique et de Cosmologie [LPSC]
dc.contributor.authorZAMPAOLO, M.
dc.contributor.authorŽUKAUSKAS, A.
dc.date.issued2020
dc.description.abstractEn<jats:title>Abstract</jats:title><jats:p>A radiochemical method for producing <jats:sup>82</jats:sup>Se sources with an ultra-low level of contamination of natural radionuclides (<jats:sup>40</jats:sup>K, decay products of <jats:sup>232</jats:sup>Th and <jats:sup>238</jats:sup>U) has been developed based on cation-exchange chromatographic purification with reverse removal of impurities. It includes chromatographic separation (purification), reduction, conditioning (which includes decantation, centrifugation, washing, grinding, and drying), and <jats:sup>82</jats:sup>Se foil production. The conditioning stage, during which highly dispersed elemental selenium is obtained by the reduction of purified selenious acid (H<jats:sub>2</jats:sub>SeO<jats:sub>3</jats:sub>) with sulfur dioxide (SO<jats:sub>2</jats:sub>) represents the crucial step in the preparation of radiopure <jats:sup>82</jats:sup>Se samples. The natural selenium (600 g) was first produced in this procedure in order to refine the method. The technique developed was then used to produce 2.5 kg of radiopure enriched selenium (<jats:sup>82</jats:sup>Se). The produced <jats:sup>82</jats:sup>Se samples were wrapped in polyethylene (12 μm thick) and radionuclides present in the sample were analyzed with the BiPo-3 detector. The radiopurity of the plastic materials (chromatographic column material and polypropylene chemical vessels), which were used at all stages, was determined by instrumental neutron activation analysis. The radiopurity of the <jats:sup>82</jats:sup>Se foils was checked by measurements with the BiPo-3 spectrometer, which confirmed the high purity of the final product. The measured contamination level for <jats:sup>208</jats:sup>Tl was 8–54 μBq/kg, and for <jats:sup>214</jats:sup>Bi the detection limit of 600 μBq/kg has been reached.</jats:p>
dc.language.isoen
dc.subject.enSelenium-82
dc.subject.enion exchange chromatography
dc.subject.enpurification
dc.subject.enmass spectrometry
dc.subject.enneutron activation analysis
dc.subject.enSuperNEMO
dc.subject.enLSM Modane
dc.subject.endouble-beta decay: (0neutrino)
dc.subject.enion: exchange
dc.subject.enselenium: nuclide
dc.subject.enselenium: production
dc.subject.enbackground: radioactivity
dc.subject.enNeutrino Ettore Majorana Observatory
dc.subject.ensulfur
dc.subject.enoxygen
dc.subject.enchemistry
dc.subject.enfabrication
dc.subject.enmeasurement methods
dc.title.enDevelopment of methods for the preparation of radiopure $^{82}$Se sources for the SuperNEMO neutrinoless double-beta decay experiment
dc.typeArticle de revue
dc.identifier.doi10.1515/ract-2019-3129
dc.subject.halPhysique [physics]
bordeaux.journalRadiochim.Acta
bordeaux.page87-97
bordeaux.volume108
bordeaux.issue2
bordeaux.peerReviewedoui
hal.identifierhal-02491286
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-02491286v1
bordeaux.COinSctx_ver=Z39.88-2004&amp;rft_val_fmt=info:ofi/fmt:kev:mtx:journal&amp;rft.jtitle=Radiochim.Acta&amp;rft.date=2020&amp;rft.volume=108&amp;rft.issue=2&amp;rft.spage=87-97&amp;rft.epage=87-97&amp;rft.au=RAKHIMOV,%20Alimardon%20V.&amp;BARABASH,%20A.S.&amp;BASHARINA-FRESHVILLE,%20A.&amp;BLOT,%20S.&amp;BONGRAND,%20M.&amp;rft.genre=article


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