FERNÉE, Mark J.; SINITO, Chiara; LOUYER, Yann; TAMARAT, Philippe; LOUNIS, Brahim

doi:10.1088/0957-4484/24/46/465703

Metadatos

Mostrar el registro completo del ítem

Licencia de uso del documento

http://creativecommons.org/licenses/by-nc/

FERNÉE, Mark J.
lp2n-01,lp2n-12

SINITO, Chiara
lp2n-01,lp2n-12

LOUYER, Yann
Laboratoire Ondes et Matière d'Aquitaine [LOMA]

Idioma

Article de revue

Este ítem está publicado en

Nanotechnology. 2013-10-24, vol. 24, p. 465703 (1-5)

Institute of Physics

Resumen en inglés

Measurements of the emission linewidth of single nanocrystals are usually limited by spectral diffusion. At cryogenic temperatures, the origin of this instability was revealed to be photo-induced, suggesting that the spectral peak position may be stable in the limit of vanishing optical excitation. Here we test this stability using resonant photoluminescence excitation and find there is persistent spectral broadening, which ultimately limits the emission linewidth in these materials. The spectral broadening is shown to be consistent with spontaneous fluctuations of the local electrostatic field within the disordered environment surrounding the nanocrystal.< Leer menos

Palabras clave en inglés

single molecule spectroscopy- spectral diffusion

band edge exciton

semiconductor nanocrystals

Metadatos

Compartir este ítem

Licencia de uso del documento

The ultimate limit to the emission linewidth of single nanocrystals

Idioma

Este ítem está publicado en

Resumen en inglés

Palabras clave en inglés

URI

DOI

Orígen

Centros de investigación