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Formation and thermo-assisted stabilization of luminescent silver clusters in photosensitive glasses

hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorBOURHIS, Kevin
hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
dc.contributor.authorROYON, Arnaud
hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
dc.contributor.authorPAPON, Gautier
hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
dc.contributor.authorBELLEC, Matthieu
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorPETIT, Yannick
hal.structure.identifierLaboratoire Ondes et Matière d'Aquitaine [LOMA]
dc.contributor.authorCANIONI, Lionel
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorDUSSAUZE, Marc
hal.structure.identifierInstitut des Sciences Moléculaires [ISM]
dc.contributor.authorRODRIGUEZ, Vincent
hal.structure.identifierLaboratoire de Chimie de la Matière Condensée de Paris (site ENSCP) [LCMCP (site ENSCP)]
dc.contributor.authorBINET, Laurent
hal.structure.identifierLaboratoire de Chimie de la Matière Condensée de Paris (site ENSCP) [LCMCP (site ENSCP)]
dc.contributor.authorCAURANT, Daniel
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorTRÉGUER-DELAPIERRE, Mona
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorVIDEAU, Jean-Jacques
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorCARDINAL, Thierry
dc.date.created2012-10-31
dc.date.issued2013
dc.identifier.issn0025-5408
dc.description.abstractEnVarious photo-induced silver luminescent centres were obtained in photosensitive zinc and phosphate glasses containing silver ions after exposure to gamma or ultraviolet nanosecond pulsed-laser radiation. Gamma-irradiation of the glasses results mainly in the formation within the glass of electron-trapped and hole-trapped silver centres as evidenced by optical absorption, luminescence and electron spin resonance spectroscopies. For the highest irradiation doses silver clusters are obtained. Under ultraviolet nanosecond pulsed-laser exposure similar species are generated along the beam propagation direction as proven by the analogous optical and luminescence signatures. In this case for high irradiation doses few silver clusters are created. The evolution of the luminescence spectra with respect to the temperature and to the duration of the heat treatment after ultraviolet nanosecond pulsed-laser irradiation evidences the presence of potential barriers determining the stability limits of some species such as the Ag2+ hole-trapped centres or the Agmx+ clusters composed of silver ions and silver atoms. A heat treatment of several hundreds of degrees is identified as a the key parameter for tailoring the optical properties and controlling the formation of Agmx+ clusters in the photosensitive glasses.
dc.description.sponsorshipFemtosecond Laser Interaction and Nanostructuring - ANR-10-BLAN-0946
dc.language.isoen
dc.publisherElsevier
dc.rights.urihttp://creativecommons.org/licenses/by-nc/
dc.title.enFormation and thermo-assisted stabilization of luminescent silver clusters in photosensitive glasses
dc.typeArticle de revue
dc.identifier.doi10.1016/j.materresbull.2013.01.003
dc.subject.halChimie/Matériaux
bordeaux.journalMaterials Research Bulletin
bordeaux.page1637-1644
bordeaux.volume48
bordeaux.issue4
bordeaux.peerReviewedoui
hal.identifierhal-00809461
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-00809461v1
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