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Rational design of layered oxide materials for sodium-ion batteries

hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorZHAO, Chenglong
hal.structure.identifierShenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene Center
hal.structure.identifierSchool of Materials Science and Engineering
dc.contributor.authorWANG, Qidi
hal.structure.identifierDepartment of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138
dc.contributor.authorYAO, Zhenpeng
hal.structure.identifierState Key Laboratory for Surface Physics
dc.contributor.authorWANG, Jianling
hal.structure.identifierDepartment of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138
dc.contributor.authorSÁNCHEZ-LENGELING, Benjamín
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorDING, Feixiang
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorQI, Xingguo
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorLU, Yaxiang
hal.structure.identifierState Key Laboratory for Surface Physics
dc.contributor.authorBAI, Xuedong
hal.structure.identifierShenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene Center
dc.contributor.authorLI, Baohua
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorLI, Hong
hal.structure.identifierDepartment of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138
hal.structure.identifierDepartment of Chemistry and Department of Computer Science
dc.contributor.authorASPURU-GUZIK, Alan
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
dc.contributor.authorHUANG, Xuejie
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorDELMAS, Claude
hal.structure.identifierDepartment of Radiation Science and Technology [Delft] [RST]
dc.contributor.authorWAGEMAKER, Marnix
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
dc.contributor.authorCHEN, Liquan
hal.structure.identifierBeijing Key Laboratory for New Energy Materials and Devices
hal.structure.identifierCenter of Materials Science and Optoelectronics Engineering
hal.structure.identifierYangtze River Delta Physics Research Center
dc.contributor.authorHU, Yong-Sheng
dc.date.issued2020
dc.identifier.issn0036-8075
dc.description.abstractEnSodium-ion batteries have captured widespread attention for grid-scale energy storage owing to the natural abundance of sodium. The performance of such batteries is limited by available electrode materials, especially for sodium-ion layered oxides, motivating the exploration of high compositional diversity. How the composition determines the structural chemistry is decisive for the electrochemical performance but very challenging to predict, especially for complex compositions. We introduce the “cationic potential” that captures the key interactions of layered materials and makes it possible to predict the stacking structures. This is demonstrated through the rational design and preparation of layered electrode materials with improved performance. As the stacking structure determines the functional properties, this methodology offers a solution toward the design of alkali metal layered oxides.
dc.language.isoen
dc.publisherAmerican Association for the Advancement of Science (AAAS)
dc.title.enRational design of layered oxide materials for sodium-ion batteries
dc.typeArticle de revue
dc.identifier.doi10.1126/science.aay9972
dc.subject.halChimie/Matériaux
bordeaux.journalScience
bordeaux.page708-711
bordeaux.volume370
bordeaux.issue6517
bordeaux.peerReviewedoui
hal.identifierhal-02992595
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-02992595v1
bordeaux.COinSctx_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.jtitle=Science&rft.date=2020&rft.volume=370&rft.issue=6517&rft.spage=708-711&rft.epage=708-711&rft.eissn=0036-8075&rft.issn=0036-8075&rft.au=ZHAO,%20Chenglong&WANG,%20Qidi&YAO,%20Zhenpeng&WANG,%20Jianling&S%C3%81NCHEZ-LENGELING,%20Benjam%C3%ADn&rft.genre=article


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