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Enhanced near-ambient temperature energy storage and electrocaloric effect in the lead-free BaTi0.89Sn0.11O3 ceramic synthesized by sol–gel method

hal.structure.identifierLaboratoire des Matériaux Innovants, Energie et Développement Durable [Marrakech] [IMED-Lab ]
dc.contributor.authorZAHID, Marwa
hal.structure.identifierLaboratoire des Matériaux Innovants, Energie et Développement Durable [Marrakech] [IMED-Lab ]
hal.structure.identifierLaboratoire de Physique de la Matière Condensée - UR UPJV 2081 [LPMC]
dc.contributor.authorHADOUCH, Youness
hal.structure.identifierLaboratoire des Matériaux Innovants, Energie et Développement Durable [Marrakech] [IMED-Lab ]
dc.contributor.authorAMJOUD, M’barek
hal.structure.identifierLaboratoire des Matériaux Innovants, Energie et Développement Durable [Marrakech] [IMED-Lab ]
hal.structure.identifierLaboratoire de Physique de la Matière Condensée - UR UPJV 2081 [LPMC]
dc.contributor.authorMEZZANE, Daoud
hal.structure.identifierInstitut de Chimie de la Matière Condensée de Bordeaux [ICMCB]
dc.contributor.authorGOUNÉ, Mohamed
hal.structure.identifierInstitut des Matériaux, de Microélectronique et des Nanosciences de Provence [IM2NP]
dc.contributor.authorHOUMMADA, Khalid
hal.structure.identifierLaboratoire des Matériaux Innovants, Energie et Développement Durable [Marrakech] [IMED-Lab ]
dc.contributor.authorALIMOUSSA, Abdelhadi
hal.structure.identifierFaculty of Physics, Southern Federal University
dc.contributor.authorRAZUMNAYA, Anna
hal.structure.identifierJozef Stefan Institute [Ljubljana] [IJS]
dc.contributor.authorROŽIČ, Brigita
hal.structure.identifierJozef Stefan Institute [Ljubljana] [IJS]
dc.contributor.authorKUTNJAK, Zdravko
dc.date.issued2022-04-27
dc.identifier.issn0957-4522
dc.description.abstractEnLead-free perovskite materials with high performance have high potential in clean energy storage applications and developments of electrocaloric devices. In this work, we report structural, dielectric, ferroelectric properties, energy storage and electrocaloric effectnear the ambient temperature in barium stannate titanate (BaTi 0.89 Sn 0.11 O 3, BTS 11) ceramic prepared by a sol-gel method. The formation of a single perovskite structure was confirmed using the X-ray diffraction analysis. An average grain size of 18.5µm was found by the mean of the SEM micrograph with a density of 5.91 g/cm 3 .The presence of the multiphase at very near ambient temperature was proved using temperature-dependent micro-Raman measurements and differential scanning calorimetry. The BTS 11 ceramic exhibits a high dielectric constant of 15460and a low dielectric loss (<0.055) with considerable temperature stability. Moreover, a high energy storage density of 122mJ/cm 3 was showed with an efficiency of 79%, and a maximum value of ECE (ΔT) of 0.86 K and finally, an electrocaloric responsivity (ΔT/ΔE) of 0.24 K.mm/kV under the external electricfield of 35 kV/cm near ambient temperature. The enhanced dielectric, ferroelectric and electrocaloric properties in BTS 11 ceramic makes it a great potential candidate for its uses in solid-state cooling technology and high-energy storage applications near ambient temperature.
dc.language.isoen
dc.publisherSpringer Verlag
dc.subject.enLead-free
dc.subject.ensol-gel process
dc.subject.enenergy storage
dc.subject.enelectrocaloric effect
dc.subject.enambient temperature
dc.subject.enbarium stannate titanate
dc.title.enEnhanced near-ambient temperature energy storage and electrocaloric effect in the lead-free BaTi0.89Sn0.11O3 ceramic synthesized by sol–gel method
dc.typeArticle de revue
dc.identifier.doi10.1007/s10854-022-08233-6
dc.subject.halChimie/Matériaux
bordeaux.journalJournal of Materials Science: Materials in Electronics
bordeaux.page12900-12911
bordeaux.volume33
bordeaux.issue16
bordeaux.peerReviewedoui
hal.identifierhal-03694850
hal.version1
hal.popularnon
hal.audienceInternationale
hal.origin.linkhttps://hal.archives-ouvertes.fr//hal-03694850v1
bordeaux.COinSctx_ver=Z39.88-2004&amp;rft_val_fmt=info:ofi/fmt:kev:mtx:journal&amp;rft.jtitle=Journal%20of%20Materials%20Science:%20Materials%20in%20Electronics&amp;rft.date=2022-04-27&amp;rft.volume=33&amp;rft.issue=16&amp;rft.spage=12900-12911&amp;rft.epage=12900-12911&amp;rft.eissn=0957-4522&amp;rft.issn=0957-4522&amp;rft.au=ZAHID,%20Marwa&amp;HADOUCH,%20Youness&amp;AMJOUD,%20M%E2%80%99barek&amp;MEZZANE,%20Daoud&amp;GOUN%C3%89,%20Mohamed&amp;rft.genre=article


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